Polyurethanes are major consumer plastic materials, ranking 6th in global plastics production (Delavarde, 2024) with an annual production of 16 million tons (NREL, 2020). Due to their superior mechanical properties, polyurethane polymers are ubiquitous and have been extensively used for a wide range of applications including foams, coatings, adhesives, sealants & elastomers. However, to date, the recycling of polyurethanes, especially with crosslinked networks, is an impractical, low value business due to numerous difficulties associated with reprocessing and/or repurposing these materials. Less than 20% of polyurethanes, mainly polyurethane thermoplastics, are recycled by methods such as rebonding, hydrogenation, and glycolysis. Recycling of polyurethanes is still an unattractive process from an economic standpoint.  To date, most recyclable and reprocessable polyurethane systems rely on remolding processes, which generally require high temperatures, metal catalysts, and suffer from a reduction in mechanical properties of the recycled materials relative to the pristine materials.  In order to overcome these limitations, many attempts have been undertaken including appropriate selection of catalysts insertion of other dynamic chemistries, and alternative polymerization methods.